Voices
- Michael Bell
- Lucille Bliss - Smurfette
- Bill Callaway
- Hamilton Camp
- Julie Dees
- June Foray
- Danny Goldman - Brainy Smurf
- Kip King
- Don Messick - Azrael the Cat, Papa Smurf
- Alan Oppenheimer
- Lennie Weinrib
- Frank Welker
- Paul Winchell - Gargamel
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